Ayçiçek yağı endüstrisi atık sularının koagülasyon-flokülasyon ve elektro-Fenton yöntemleriyle arıtılması
Yıl: 2021 Cilt: 36 Sayı: 1 Sayfa Aralığı: 275 - 290 Metin Dili: Türkçe DOI: 10.17341/gazimmfd.553847 İndeks Tarihi: 09-11-2022
Ayçiçek yağı endüstrisi atık sularının koagülasyon-flokülasyon ve elektro-Fenton yöntemleriyle arıtılması
Öz: Bitkisel yağların üretimi sırasında oluşan yüksek miktarda organik kirlilik içeren endüstriyel atık sular, alıcı ortamlara deşarj edilmeden önce arıtılmalıdır. Yapılan çalışmada koagülasyon-flokülasyon ve elektro- Fenton yöntemleri ve iki yöntemin ardışık işletimi ile ayçiçek yağı endüstrisi atık suyunun arıtımı gerçekleştirilmiştir. Koagülasyon-flokülasyon yöntemiyle arıtımda en uygun koagülant türü ve derişimi, flokülant derişimi ve pH’ın belirlenmesi amacıyla PACl ve Al2(SO4)3.18H2O koagülantları kullanılarak 4, 10, 16 g/L değerlerinde, flokülant olarak anyonik ticari polielektrolit kullanılarak 0,06, 0,18 ve 0,3 g/L değerlerinde ve pH 4, 6, 8 koşullarında çalışmalar gerçekleştirilmiştir. Elde edilen en uygun değerlerde (10 g/L Al2(SO4)3.18H2O, 0,06 g/L flokülant, pH 6) yapılan çalışmada %97 kimyasal oksijen ihtiyacı (KOİ) giderimine ulaşılmıştır. Elektro-Fenton yöntemi ile yapılan arıtım çalışmalarında 1, 2,5, 4 A akım şiddeti, 4,5, 9, 18 g/L FeSO4.7H2O derişimi, 32,71, 81,77, 130,84 mM H2O2 derişimi, 3, 5,5, 8 pH değerleri çalışılmış ve en uygun işletim koşulları 1 A akım şiddeti, 9 g/L FeSO4.7H2O, 130,84 mM H2O2, 6,06 H2O2/Fe2+ mol oranı ve pH 3 olarak belirlenmiştir. Bu koşullarda yapılan çalışmada %99 KOİ giderimi ve 2,37 kWh/m3 enerji tüketimi elde edilmiştir. Belirlenen en uygun işletim koşullarında ardışık koagülasyon-flokülasyon-elektro-Fenton yöntemi ile yapılan arıtımda ise 15 min sonunda %98 KOİ giderimi ve 0,48 kWh/m3 enerji tüketimi değerlerine ulaşılmış olup arıtım sonundaki KOİ değeri (183 mg/L) deşarj sınırlarının altında olduğundan deşarj edilebilir kalitede su eldesi sağlanmıştır.
Anahtar Kelime: Treatment of sunflower oil industry wastewater by coagulation-flocculation and electro- Fenton methods
Öz: High levels of organic pollutant containing industrial wastewaters which are generated during the production of vegetable oils must be treated before discharge to the receiving environments. In this work, treatment of sunflower oil industry wastewater was performed via coagulation-flocculation, electro-Fenton and sequential operation of these two methods. To determine optimum coagulant concentration, flocculant concentration and pH, coagulation-flocculation studies were carried out under 4, 10, 16 g/L PACl and Al2(SO4)3.18H2O coagulant concentrations, 0.06, 0.18, 0.3 g/L anionic commercial polyelectrolyte concentrations and 4, 6, 8 pH values, respectively. Results showed a COD removal of 97% under optimum conditions of 10 g/L Al2(SO4)3.18H2O, 0.06 g/L flocculant concentration and pH 6. Electro-Fenton studies were performed under 1, 2.5, 4 A current intensity, 4.5, 9, 18 g/L FeSO4.7H2O concentration, 32.71, 81.77, 130.84 mM H2O2 concentration, and 3, 5.5, 8 pH conditions. Optimum operating conditions for electro-Fenton method were obtained as 1 A, 9 g/L FeSO4.7H2O, 130.84 mM H2O2, 6.06 H2O2/Fe2+ molar ratio and pH 3. Treatment under optimum conditions revealed 99% COD removal and 2.37 kWh/m3 energy consumption for electro- Fenton method. Sequential coagulation-flocculation-electro-Fenton method under optimum conditions resulted in 98% COD removal and 0.48 kWh/m3 energy consumption at 15 min operation, thus the treated water is dischargeable since COD value (183 mg/L) is below discharge limits.
Anahtar Kelime: Belge Türü: Makale Makale Türü: Araştırma Makalesi Erişim Türü: Erişime Açık
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| APA | OZYURT B, CAMCIOGLU S, Karatokus T, Yuksek C, Hapoglu H (2021). Ayçiçek yağı endüstrisi atık sularının koagülasyon-flokülasyon ve elektro-Fenton yöntemleriyle arıtılması. , 275 - 290. 10.17341/gazimmfd.553847 |
| Chicago | OZYURT BARAN,CAMCIOGLU SULE,Karatokus Toprak,Yuksek Ceren,Hapoglu Hale Ayçiçek yağı endüstrisi atık sularının koagülasyon-flokülasyon ve elektro-Fenton yöntemleriyle arıtılması. (2021): 275 - 290. 10.17341/gazimmfd.553847 |
| MLA | OZYURT BARAN,CAMCIOGLU SULE,Karatokus Toprak,Yuksek Ceren,Hapoglu Hale Ayçiçek yağı endüstrisi atık sularının koagülasyon-flokülasyon ve elektro-Fenton yöntemleriyle arıtılması. , 2021, ss.275 - 290. 10.17341/gazimmfd.553847 |
| AMA | OZYURT B,CAMCIOGLU S,Karatokus T,Yuksek C,Hapoglu H Ayçiçek yağı endüstrisi atık sularının koagülasyon-flokülasyon ve elektro-Fenton yöntemleriyle arıtılması. . 2021; 275 - 290. 10.17341/gazimmfd.553847 |
| Vancouver | OZYURT B,CAMCIOGLU S,Karatokus T,Yuksek C,Hapoglu H Ayçiçek yağı endüstrisi atık sularının koagülasyon-flokülasyon ve elektro-Fenton yöntemleriyle arıtılması. . 2021; 275 - 290. 10.17341/gazimmfd.553847 |
| IEEE | OZYURT B,CAMCIOGLU S,Karatokus T,Yuksek C,Hapoglu H "Ayçiçek yağı endüstrisi atık sularının koagülasyon-flokülasyon ve elektro-Fenton yöntemleriyle arıtılması." , ss.275 - 290, 2021. 10.17341/gazimmfd.553847 |
| ISNAD | OZYURT, BARAN vd. "Ayçiçek yağı endüstrisi atık sularının koagülasyon-flokülasyon ve elektro-Fenton yöntemleriyle arıtılması". (2021), 275-290. https://doi.org/10.17341/gazimmfd.553847 |
| APA | OZYURT B, CAMCIOGLU S, Karatokus T, Yuksek C, Hapoglu H (2021). Ayçiçek yağı endüstrisi atık sularının koagülasyon-flokülasyon ve elektro-Fenton yöntemleriyle arıtılması. Gazi Üniversitesi Mühendislik Mimarlık Fakültesi Dergisi, 36(1), 275 - 290. 10.17341/gazimmfd.553847 |
| Chicago | OZYURT BARAN,CAMCIOGLU SULE,Karatokus Toprak,Yuksek Ceren,Hapoglu Hale Ayçiçek yağı endüstrisi atık sularının koagülasyon-flokülasyon ve elektro-Fenton yöntemleriyle arıtılması. Gazi Üniversitesi Mühendislik Mimarlık Fakültesi Dergisi 36, no.1 (2021): 275 - 290. 10.17341/gazimmfd.553847 |
| MLA | OZYURT BARAN,CAMCIOGLU SULE,Karatokus Toprak,Yuksek Ceren,Hapoglu Hale Ayçiçek yağı endüstrisi atık sularının koagülasyon-flokülasyon ve elektro-Fenton yöntemleriyle arıtılması. Gazi Üniversitesi Mühendislik Mimarlık Fakültesi Dergisi, vol.36, no.1, 2021, ss.275 - 290. 10.17341/gazimmfd.553847 |
| AMA | OZYURT B,CAMCIOGLU S,Karatokus T,Yuksek C,Hapoglu H Ayçiçek yağı endüstrisi atık sularının koagülasyon-flokülasyon ve elektro-Fenton yöntemleriyle arıtılması. Gazi Üniversitesi Mühendislik Mimarlık Fakültesi Dergisi. 2021; 36(1): 275 - 290. 10.17341/gazimmfd.553847 |
| Vancouver | OZYURT B,CAMCIOGLU S,Karatokus T,Yuksek C,Hapoglu H Ayçiçek yağı endüstrisi atık sularının koagülasyon-flokülasyon ve elektro-Fenton yöntemleriyle arıtılması. Gazi Üniversitesi Mühendislik Mimarlık Fakültesi Dergisi. 2021; 36(1): 275 - 290. 10.17341/gazimmfd.553847 |
| IEEE | OZYURT B,CAMCIOGLU S,Karatokus T,Yuksek C,Hapoglu H "Ayçiçek yağı endüstrisi atık sularının koagülasyon-flokülasyon ve elektro-Fenton yöntemleriyle arıtılması." Gazi Üniversitesi Mühendislik Mimarlık Fakültesi Dergisi, 36, ss.275 - 290, 2021. 10.17341/gazimmfd.553847 |
| ISNAD | OZYURT, BARAN vd. "Ayçiçek yağı endüstrisi atık sularının koagülasyon-flokülasyon ve elektro-Fenton yöntemleriyle arıtılması". Gazi Üniversitesi Mühendislik Mimarlık Fakültesi Dergisi 36/1 (2021), 275-290. https://doi.org/10.17341/gazimmfd.553847 |
