Foto-Kataliz İçin Verimli Duyarlılaştırma Mekanizmasına Sahip Ag@HfO2 Çekirdek-Kabuk Nanoyapıların Tasarımı

MEHMET YILMAZ (ATATÜRK Ü. KAZIM KARABEKİR EĞİTİM F. MATEMATİK VE FEN BİLİMLERİ EĞİTİMİ B. FEN BİLGİSİ EĞİTİMİ ABD)
ŞAKİR AYDOĞAN (ATATÜRK Ü.)
NURTAÇ CANPOLAT, (ATATÜRK Ü. KAZIM KARABEKİR EĞİTİM F. KİMYA EĞİTİMİ B.)
ADEM KOÇYİĞİT, (BİLECİK ŞEYH EDEBALİ Ü. MESLEK Y.O.)
ERMAN ERDOĞAN (BİLECİK ŞEYH EDEBALİ Ü. MESLEK Y.O.)
11 0

Proje Grubu: MFAG Sayfa Sayısı: 85 Proje No: 122F075 Proje Bitiş Tarihi: 15.06.2023 Metin Dili: Türkçe DOI: 122F075 İndeks Tarihi: 12-03-2024

Foto-Kataliz İçin Verimli Duyarlılaştırma Mekanizmasına Sahip Ag@HfO2 Çekirdek-Kabuk Nanoyapıların Tasarımı

Öz:
Nüfus artışıyla birlikte yoğunlaşan tarımsal ve endüstriyel faaliyetlerin sonucunda ortaya çıkan atıklar içme sularında ağır metallerin veya organik kirleticilerin artmasına neden olmaktadır. Her geçen gün temiz suya olan ihtiyacın artışı ve küresel ısınmanın su kıtlığını tetiklemesi sulardaki kirlenmenin giderimini son derece önemli hale getirmektedir. Bu bağlamda, tekstilden ilaç sanayine kadar geniş bir uygulama alanına sahip olan organik kirleticilerden olan sentetik boyaların atık sulardan temizlenmesi hayati önem arz etmektedir. Bu çalışma kapsamında sulardaki sentetik boya kirliliği problemine odaklanılmıştır. Bu amaca yönelik olarak, yeni bir katalizör olarak sunulan Ag@HfO2 çekirdek-kabuk nanoyapılarının yaygın endüstriyel sentetik kirleticiler arasında yer alan katyonik boyalardan Rodamin B (RhB), metilen mavisi (MB) ve direkt kırmızı-23 (DR-23) kirleticilerinin fotokatalitik bozunmasındaki performansları incelenmiştir. Sentezlenen yapıların X-ışınları kırınım difraktometresi (XRD), geçirmeli elektron mikroskopu (TEM) X-ışınları fotoelektron spektroskopisi, UV-Vis ve fotolüminesans spektroskopileri ile karakterizasyonu Ag@HfO2 çekirdek-kabuk nanoyapılarının başarılı bir şekilde sentezlendiğini ortaya konmuştur. Daha sonra sentezlenen Ag@HfO2 çekirdek-kabuk nanoyapılarının fotodegredasyon için uygunluğu test edilmiştir. Fotokatalitik ölçümler, ilgili boyaların hem UV bölgede hem de görünür bölgede yüksek verim ile giderebildiğini göstermiştir. Elde edilen sonuçlara dayalı olarak Ag@HfO2 çekirdek-kabuk nanoyapılarının çevre sağlığı bakımından oldukça önemli görülen bir problemin çözümüne katkı sağlayacağı söylenebilir.
Anahtar Kelime: Fotokataliz HfO2 nanoparçacıklar Ag nanoparçacıklar Ag@HfO2 çekirdek-kabuk nanoyapılar

Design of Ag@HfO2 Core-Shell Nanostructures with Efficient Sensitization Mechanism for Photocatalysis

Öz:
Waste generated by agricultural and industrial activities, which are intensifying as the population grows, cause an increase in heavy metals or organic pollutants in drinking water. With the demand for water increasing day by day and global warming threatening to make water scarce, the need to remove pollution from water is paramount. In this context, it is vital to remove synthetic dyes from wastewater, which are organic pollutants with a wide range of applications from textiles to pharmaceuticals. This study focuses on the problem of synthetic dyes in water. To this end, the performance of Ag@HfO2 core-shell nanostructures, presented as a new catalyst, was investigated in the photocatalytic degradation of the cationic dyes Rhodamine B (RhB), Methylene Blue (MB) and Direct Red 23 (DR-23), which are among the most common industrial synthetic pollutants. The synthesized structures were characterized by X-ray diffractometry (XRD), transmission electron microscopy (TEM), X-ray photoelectron spectroscopy, UV-Vis and photoluminescence spectroscopy, and it was revealed that Ag@HfO2 core-shell nanostructures were successfully synthesized. Then, the suitability of the synthesized Ag@HfO2 core-shell nanostructures for photo-degradation was found to be able to remove dyes related to photocatalytic measurements with high efficiency both in the UV region and the visible region. It is predicted that the results will contribute to the solution of a problem that is considered very important in terms of environmental health.
Anahtar Kelime: Fotokataliz HfO2 nanoparçacıklar Ag nanoparçacıklar Ag@HfO2 çekirdek-kabuk nanoyapılar

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APA Yilmaz M, aydogan s, CANPOLAT N, A, Erdoğan E (2023). Foto-Kataliz İçin Verimli Duyarlılaştırma Mekanizmasına Sahip Ag@HfO2 Çekirdek-Kabuk Nanoyapıların Tasarımı. , 0 - 85. 122F075
Chicago Yilmaz Mehmet,aydogan sakir,CANPOLAT NURTAÇ, Adem,Erdoğan Erman Foto-Kataliz İçin Verimli Duyarlılaştırma Mekanizmasına Sahip Ag@HfO2 Çekirdek-Kabuk Nanoyapıların Tasarımı. (2023): 0 - 85. 122F075
MLA Yilmaz Mehmet,aydogan sakir,CANPOLAT NURTAÇ, Adem,Erdoğan Erman Foto-Kataliz İçin Verimli Duyarlılaştırma Mekanizmasına Sahip Ag@HfO2 Çekirdek-Kabuk Nanoyapıların Tasarımı. , 2023, ss.0 - 85. 122F075
AMA Yilmaz M,aydogan s,CANPOLAT N, A,Erdoğan E Foto-Kataliz İçin Verimli Duyarlılaştırma Mekanizmasına Sahip Ag@HfO2 Çekirdek-Kabuk Nanoyapıların Tasarımı. . 2023; 0 - 85. 122F075
Vancouver Yilmaz M,aydogan s,CANPOLAT N, A,Erdoğan E Foto-Kataliz İçin Verimli Duyarlılaştırma Mekanizmasına Sahip Ag@HfO2 Çekirdek-Kabuk Nanoyapıların Tasarımı. . 2023; 0 - 85. 122F075
IEEE Yilmaz M,aydogan s,CANPOLAT N, A,Erdoğan E "Foto-Kataliz İçin Verimli Duyarlılaştırma Mekanizmasına Sahip Ag@HfO2 Çekirdek-Kabuk Nanoyapıların Tasarımı." , ss.0 - 85, 2023. 122F075
ISNAD Yilmaz, Mehmet vd. "Foto-Kataliz İçin Verimli Duyarlılaştırma Mekanizmasına Sahip Ag@HfO2 Çekirdek-Kabuk Nanoyapıların Tasarımı". (2023), 0-85. https://doi.org/122F075
APA Yilmaz M, aydogan s, CANPOLAT N, A, Erdoğan E (2023). Foto-Kataliz İçin Verimli Duyarlılaştırma Mekanizmasına Sahip Ag@HfO2 Çekirdek-Kabuk Nanoyapıların Tasarımı. , 0 - 85. 122F075
Chicago Yilmaz Mehmet,aydogan sakir,CANPOLAT NURTAÇ, Adem,Erdoğan Erman Foto-Kataliz İçin Verimli Duyarlılaştırma Mekanizmasına Sahip Ag@HfO2 Çekirdek-Kabuk Nanoyapıların Tasarımı. (2023): 0 - 85. 122F075
MLA Yilmaz Mehmet,aydogan sakir,CANPOLAT NURTAÇ, Adem,Erdoğan Erman Foto-Kataliz İçin Verimli Duyarlılaştırma Mekanizmasına Sahip Ag@HfO2 Çekirdek-Kabuk Nanoyapıların Tasarımı. , 2023, ss.0 - 85. 122F075
AMA Yilmaz M,aydogan s,CANPOLAT N, A,Erdoğan E Foto-Kataliz İçin Verimli Duyarlılaştırma Mekanizmasına Sahip Ag@HfO2 Çekirdek-Kabuk Nanoyapıların Tasarımı. . 2023; 0 - 85. 122F075
Vancouver Yilmaz M,aydogan s,CANPOLAT N, A,Erdoğan E Foto-Kataliz İçin Verimli Duyarlılaştırma Mekanizmasına Sahip Ag@HfO2 Çekirdek-Kabuk Nanoyapıların Tasarımı. . 2023; 0 - 85. 122F075
IEEE Yilmaz M,aydogan s,CANPOLAT N, A,Erdoğan E "Foto-Kataliz İçin Verimli Duyarlılaştırma Mekanizmasına Sahip Ag@HfO2 Çekirdek-Kabuk Nanoyapıların Tasarımı." , ss.0 - 85, 2023. 122F075
ISNAD Yilmaz, Mehmet vd. "Foto-Kataliz İçin Verimli Duyarlılaştırma Mekanizmasına Sahip Ag@HfO2 Çekirdek-Kabuk Nanoyapıların Tasarımı". (2023), 0-85. https://doi.org/122F075
Sayfa Oluşturulma Tarihi
24-04-2024 10:56

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TÜBİTAK ULAKBİM TR Dizin

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